Masterminds are considered geniuses among geniuses; in other words, they are among the most intelligent beings in existence and are characterized by a personality in which they will plan things to amazing lengths and always have a backup plan. They are often extremely difficult to catch or defeat due to their incredibly complex schemes.
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- Abbott Hayes
- Abigail Williams (Murdered: Soul Suspect)
- Ace (The Powerpuff Girls)
- Adam (Buffyverse)
- Adam Barlow
- Adolf Hitler (The Twilight Zone)
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- Agatha Trunchbull
- Agent Kruger
- Agent Orange (Marvel Cinematic Universe)
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- Aggregor
- Ajax (X-Men Movies)
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- Akihiro Kurata
- Aku
- Al-G Rhythm
- Albert Wesker
- Alec Trevelyan
- Aleema Keto
- Alejandro Gutierrez
- Alex Wesker
- Alonzo Harris
- Alternates
- Amon Goeth
- Andy Hunter
- Anton LaVey (American Horror Story)
- April Troost
- Archibald Snatcher
- Aresia
- Ariel Augustus
- Arjen Rudd
- Arthur (Wreck-It Ralph)
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- Arthur Slugworth (Wonka)
- Ash Landers
- Auric Goldfinger
- AUTO
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B
- Babidi
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- Bane (The Dark Knight Rises)
- Baron Corbin
- Barracuda (Marvel)
- Belle Bottom
- Belle Fontiere
- Bibidi
- Big Jack Horner
- Bill Cipher
- Bill Sykes
- Billy Loomis
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- Boingo
- Bomb Voyage
- Boogie Man
- Botticelli Remorso
- Bowser
- Bowser (The Super Mario Bros. Movie)
- Brainiac
- Bree Blackburn
- Bria
- Brokenstar
- Broodwing
- Burt Hartman
- Byleth Eisner
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- Captain Armando Salazar
- Captain Chantel DuBois
- Captain Cold
- Captain Kuro
- Carl King (Emmerdale)
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- Caturamon
- Chalis
- Chameleon (T.U.F.F. Puppy)
- Chaos
- Charles Rane
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- Chester Hardwick
- Chester V
- Chucky
- Circus Baby
- Claudius
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- Clone trooper
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- Colleen McCandless
- Constantine
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- Crocodile (One Piece)
- Cruella De Vil (Disney)
- Cyrus Grissom
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- D-Reaper
- Dag
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- Dark Samus
- Darkonda
- Darkseid (DC Animated Universe)
- Darth Maul
- Darth Sidious
- Darth Vader
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- David Hagan
- Davros
- Deviot
- Dick Finley
- Diesel 10
- Dio Brando
- Dirty Rat
- Doctor Doom (2015 Film)
- Doctor Octopus (Spider-Man Films)
- Doctor Octopus(Marvel Comics)
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- Dollmaker
- Dr Evil
- Dr. Alexander Isaacs
- Dr. Blowhole
- Dr. Carl Mortner
- Dr. Charles Nichols
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- Dr. Henry Miller
- Dr. Ivo "Eggman" Robotnik
- Dr. Kulik
- Dr. Nefarious Tropy (original)
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- Dr. Robotnik (Live-Action)
- Drago Bludvist
- Drago's Bewilderbeast
- Dreadpool
- Duchess (Foster's Home for Imaginary Friends)
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- Edgar The Bug
- Eggman Nega
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- Ein
- El Macho
- Elder Princess Shroob
- Eleanor (Fazbear Frights)
- Elliot Carver
- Emilio Largo
- Emperor Palpatine
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- Ernst Stavro Blofeld
- Ernst Stavro Blofeld (Reboot Series)
- Esther Coleman
- Eustace Strych
- Evelyn Deavor
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G
- G-Man
- Gabriel (The Mandela Catalogue)
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- Gargamel (The Smurfs Film Series)
- Gary Windass
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- General Armitage Hux
- General Hux (LEGO)
- General Kalani
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- General Shanker
- General Zod
- Glichtrap
- Goku Black
- Gold Toothed Doctor
- Gollum
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- Grand High Witch
- Grand Moff Tarkin
- Grandfather
- Green Goblin (Sam Raimi trilogy/Spider-Man: No Way Home)
- Green Goblin (The Spectacular Spider Man)
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- Gul'dan
- Gunmar
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